The singer is currently on a farewell tour following his recent announcement that he is suffering from Alzheimer's disease.
"I think it would surprise you how good it would sound, me and Cee Lo together," Shelton says.
The guitarist is the country group's last bachelor, and he'll walk down the aisle with his fiancee on February 4.
Pickler admits her upbringing was tough, and she used her anguish to help her write the track "Mother's Day" for her album 100 Proof.
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